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2009


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Full phase and amplitude control in computer-generated holography

Fratz, M., Fischer, P., Giel, D. M.

OPTICS LETTERS, 34(23):3659-3661, 2009 (article)

Abstract
We report what we believe to be the first realization of a computer-generated complex-valued hologram recorded in a single film of photoactive polymer. Complex-valued holograms give rise to a diffracted optical field with control over its amplitude and phase. The holograms are generated by a one-step direct laser writing process in which a spatial light modulator (SLM) is imaged onto a polymer film. Temporal modulation of the SLM during exposure controls both the strength of the induced birefringence and the orientation of the fast axis. We demonstrate that complex holograms can be used to impart arbitrary amplitude and phase profiles onto a beam and thereby open new possibilities in the control of optical beams. (C) 2009 Optical Society of America

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2009


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Digital polarization holograms with defined magnitude and orientation of each pixel’s birefringence

Fratz, M., Giel, D. M., Fischer, P.

OPTICS LETTERS, 34(8):1270-1272, 2009 (article)

Abstract
A new form of digital polarization holography is demonstrated that permits both the amplitude and the phase of a diffracted beam to be independently controlled. This permits two independent intensity images to be stored in the same hologram. To fabricate the holograms, a birefringence with defined retardance and orientation of the fast axis is recorded into a photopolymer film. The holograms are selectively read out by choosing the polarization state of the read beam. Polarization holograms of this kind increase the data density in holographic data storage and allow higher quality diffractive optical elements to be written. (C) 2009 Optical Society of America

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Controlled Propulsion of Artificial Magnetic Nanostructured Propellers

Ghosh, A., Fischer, P.

NANO LETTERS, 9(6):2243-2245, 2009, Featured highlight ‘Nanotechnology: The helix that delivers’ Nature 459, 13 (2009). (article)

Abstract
For biomedical applications, such as targeted drug delivery and microsurgery, it is essential to develop a system of swimmers that can be propelled wirelessly in fluidic environments with good control. Here, we report the construction and operation of chiral colloidal propellers that can be navigated in water with micrometer-level precision using homogeneous magnetic fields. The propellers are made via nanostructured surfaces and can be produced in large numbers. The nanopropellers can carry chemicals, push loads, and act as local probes in rheological measurements.

Featured highlight ‘Nanotechnology: The helix that delivers’ Nature 459, 13 (2009).

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Video - Nanospropellers DOI [BibTex]

Video - Nanospropellers DOI [BibTex]


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Absolute Asymmetric Reduction Based on the Relative Orientation of Achiral Reactants

Kuhn, A., Fischer, P.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 48(37):6857-6860, 2009 (article)

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DOI [BibTex]

DOI [BibTex]


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Magnetic mobile micro-robots

Pawashe, C., Floyd, S., Sitti, M.

7eme Journees Nationales de la Recherche en Robotique, 2009 (article)

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Gecko-Inspired Directional and Controllable Adhesion

Murphy, M. P., Aksak, B., Sitti, M.

Small, 5(2):170-175, WILEY-VCH Verlag, 2009 (article)

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Project Page [BibTex]

Project Page [BibTex]


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Multiple magnetic microrobot control using electrostatic anchoring

Pawashe, C., Floyd, S., Sitti, M.

Applied Physics Letters, 94(16):164108, AIP, 2009 (article)

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Characterization of bacterial actuation of micro-objects

Behkam, B., Sitti, M.

In Robotics and Automation, 2009. ICRA’09. IEEE International Conference on, pages: 1022-1027, 2009 (inproceedings)

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Wet self-cleaning of biologically inspired elastomer mushroom shaped microfibrillar adhesives

Kim, S., Cheung, E., Sitti, M.

Langmuir, 25(13):7196-7199, ACS Publications, 2009 (article)

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Compliant footpad design analysis for a bio-inspired quadruped amphibious robot

Park, H. S., Sitti, M.

In Intelligent Robots and Systems, 2009. IROS 2009. IEEE/RSJ International Conference on, pages: 645-651, 2009 (inproceedings)

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A novel artificial hair receptor based on aligned PVDF micro/nano fibers

Weiting, Liu, Bilsay, Sumer, Cesare, Stefanini, Arianna, Menciassi, Fei, Li, Dajing, Chen, Paolo, Dario, Metin, Sitti, Xin, Fu

In Robotics and Biomimetics, 2008. ROBIO 2008. IEEE International Conference on, pages: 49-54, 2009 (inproceedings)

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Robot ceiling climbers harness new tricks

Marks, Paul

New Scientist, 202(2705):18-19, Reed Business Information, 2009 (article)

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Waalbot: Agile climbing with synthetic fibrillar dry adhesives

Murphy, M. P., Sitti, M.

In Robotics and Automation, 2009. ICRA’09. IEEE International Conference on, pages: 1599-1600, 2009 (inproceedings)

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Biologically-Inspired Patterned and Coated Adhesives for Medical Devices

Glass, P, Chung, H, Lee, C, Tworkoski, E, Washburn, NR, Sitti, M

Journal of Medical Devices, 3(2):027537, American Society of Mechanical Engineers, 2009 (article)

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Modeling and experimental characterization of an untethered magnetic micro-robot

Pawashe, C., Floyd, S., Sitti, M.

The International Journal of Robotics Research, 28(8):1077-1094, Sage Publications, 2009 (article)

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Towards automated nanoassembly with the atomic force microscope: A versatile drift compensation procedure

Krohs, F., Onal, C., Sitti, M., Fatikow, S.

Journal of Dynamic Systems, Measurement, and Control, 131(6):061106, American Society of Mechanical Engineers, 2009 (article)

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Enhanced adhesion by gecko-inspired hierarchical fibrillar adhesives

Murphy, M. P., Kim, S., Sitti, M.

ACS applied materials \& interfaces, 1(4):849-855, American Chemical Society, 2009 (article)

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Project Page [BibTex]

Project Page [BibTex]


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Miniature devices: Voyage of the microrobots

Sitti, M.

Nature, 458(7242):1121-1122, Nature Publishing Group, 2009 (article)

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Piezoelectric ultrasonic resonant micromotor with a volume of less than 1 mm 3 for use in medical microbots

Watson, B., Friend, J., Yeo, L., Sitti, M.

In Robotics and Automation, 2009. ICRA’09. IEEE International Conference on, pages: 2225-2230, 2009 (inproceedings)

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Dynamic modeling and analysis of pitch motion of a basilisk lizard inspired quadruped robot running on water

Park, H. S., Floyd, S., Sitti, M.

In Robotics and Automation, 2009. ICRA’09. IEEE International Conference on, pages: 2655-2660, 2009 (inproceedings)

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Dry spinning based spinneret based tunable engineered parameters (STEP) technique for controlled and aligned deposition of polymeric nanofibers

Nain, A. S., Sitti, M., Jacobson, A., Kowalewski, T., Amon, C.

Macromolecular rapid communications, 30(16):1406-1412, WILEY-VCH Verlag, 2009 (article)

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Two-dimensional contact and noncontact micromanipulation in liquid using an untethered mobile magnetic microrobot

Floyd, S., Pawashe, C., Sitti, M.

IEEE Transactions on Robotics, 25(6):1332-1342, IEEE, 2009 (article)

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A scaled bilateral control system for experimental one-dimensional teleoperated nanomanipulation

Onal, C. D., Sitti, M.

The International Journal of Robotics Research, 28(4):484-497, Sage Publications, 2009 (article)

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A Swallowable Tethered Capsule Endoscope for Diagnosing Barrett’s Esophagus

Glass, P., Sitti, M., Pennathur, A., Appasamy, R.

Gastrointestinal Endoscopy, 69(5):AB106, Mosby, 2009 (article)

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Project Page [BibTex]

Project Page [BibTex]


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A miniature ceiling walking robot with flat tacky elastomeric footpads

Unver, O., Sitti, M.

In Robotics and Automation, 2009. ICRA’09. IEEE International Conference on, pages: 2276-2281, 2009 (inproceedings)

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Adhesion of biologically inspired polymer microfibers on soft surfaces

Cheung, E., Sitti, M.

Langmuir, 25(12):6613-6616, ACS Publications, 2009 (article)

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Dangling chain elastomers as repeatable fibrillar adhesives

Sitti, M., Cusick, B., Aksak, B., Nese, A., Lee, H., Dong, H., Kowalewski, T., Matyjaszewski, K.

ACS applied materials \& interfaces, 1(10):2277-2287, American Chemical Society, 2009 (article)

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Reversible dry micro-fibrillar adhesives with thermally controllable adhesion

Kim, S., Sitti, M., Xie, T., Xiao, X.

Soft Matter, 5(19):3689-3693, Royal Society of Chemistry, 2009 (article)

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Project Page [BibTex]

Project Page [BibTex]


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Biologically Inspired Polymer Microfibrillar Arrays for Mask Sealing

Cheung, E., Aksak, B., Sitti, M.

CARNEGIE-MELLON UNIV PITTSBURGH PA, 2009 (techreport)

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Tankbot: A miniature, peeling based climber on rough and smooth surfaces

Unver, O., Sitti, M.

In Robotics and Automation, 2009. ICRA’09. IEEE International Conference on, pages: 2282-2287, 2009 (inproceedings)

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Automated 2-D nanoparticle manipulation with an atomic force microscope

Onal, C. D., Ozcan, O., Sitti, M.

In Robotics and Automation, 2009. ICRA’09. IEEE International Conference on, pages: 1814-1819, 2009 (inproceedings)

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Enhanced reversible adhesion of dopamine methacrylamide-coated elastomer microfibrillar structures under wet conditions

Glass, P., Chung, H., Washburn, N. R., Sitti, M.

Langmuir, 25(12):6607-6612, ACS Publications, 2009 (article)

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Project Page [BibTex]

Project Page [BibTex]


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Microparticle manipulation using multiple untethered magnetic micro-robots on an electrostatic surface

Floyd, S., Pawashe, C., Sitti, M.

In Intelligent Robots and Systems, 2009. IROS 2009. IEEE/RSJ International Conference on, pages: 528-533, 2009 (inproceedings)

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2003


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New electro-optic effect: Sum-frequency generation from optically active liquids in the presence of a dc electric field

Fischer, P., Buckingham, A., Beckwitt, K., Wiersma, D., Wise, F.

PHYSICAL REVIEW LETTERS, 91(17), 2003 (article)

Abstract
We report the observation of sum-frequency signals that depend linearly on an applied electrostatic field and that change sign with the handedness of an optically active solute. This recently predicted chiral electro-optic effect exists in the electric-dipole approximation. The static electric field gives rise to an electric-field-induced sum-frequency signal (an achiral third-order process) that interferes with the chirality-specific sum-frequency at second order. The cross-terms linear in the electrostatic field constitute the effect and may be used to determine the absolute sign of second- and third-order nonlinear-optical susceptibilities in isotropic media.

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DOI [BibTex]

2003


DOI [BibTex]


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Chiral and achiral contributions to sum-frequency generation from optically active solutions of binaphthol

Fischer, P., Wise, F., Albrecht, A.

JOURNAL OF PHYSICAL CHEMISTRY A, 107(40):8232-8238, 2003 (article)

Abstract
The nonlinear sum- and difference-frequency generation spectroscopies can be probes of molecular chirality in optically active systems. We present a tensorial analysis of the chirality-specific electric-dipolar sum-frequency-generation susceptibility and the achiral electric-quadrupolar and magnetic-dipolar nonlinearities at second order in isotropic media. The chiral and achiral contributions to the sum-frequency signal from the bulk of optically active solutions of 1,1'-bi-2-naphthol (2,2'-dehydroxy-1,1'-binaphthyl) can be distinguished, and the former dominates. Ab initio computations reveal the dramatic resonance enhancement that the isotropic component of the electric-dipolar three-wave mixing hyperpolarizability experiences. Away from resonance its magnitude rapidly decreases, as-unlike the vector component-it is zero in the static limit. The dispersion of the first hyperpolarizability is computed by a configuration interaction singles sum-over-states approach with explicit regard to the Franck-Condon active vibrational substructure for all resonant electronic states.

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DOI [BibTex]

DOI [BibTex]


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Synthetic gecko foot-hair micro/nano-structures as dry adhesives

Sitti, M., Fearing, R. S.

Journal of adhesion science and technology, 17(8):1055-1073, Taylor & Francis Group, 2003 (article)

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Project Page [BibTex]

Project Page [BibTex]


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Teleoperated touch feedback from the surfaces at the nanoscale: modeling and experiments

Sitti, M., Hashimoto, H.

IEEE/ASME transactions on mechatronics, 8(2):287-298, IEEE, 2003 (article)

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High aspect ratio polymer micro/nano-structure manufacturing using nanoembossing, nanomolding and directed self-assembly

Sitti, M.

In ASME 2003 International Mechanical Engineering Congress and Exposition, pages: 293-297, 2003 (inproceedings)

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Nsf workshop on future directions in nano-scale systems, dynamics and control

Sitti, M.

In Automatic Control Conference (ACC), 2003 (inproceedings)

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3-D nano-fiber manufacturing by controlled pulling of liquid polymers using nano-probes

Nain, A. S., Sitti, M.

In Nanotechnology, 2003. IEEE-NANO 2003. 2003 Third IEEE Conference on, 1, pages: 60-63, 2003 (inproceedings)

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Scaled teleoperation system for nano-scale interaction and manipulation

Sitti, M., Aruk, B., Shintani, H., Hashimoto, H.

Advanced Robotics, 17(3):275-291, Taylor & Francis Group, 2003 (article)

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Manufacturing of two and three-dimensional micro/nanostructures by integrating optical tweezers with chemical assembly

Castelino, K., Satyanarayana, S., Sitti, M.

In Nanotechnology, 2003. IEEE-NANO 2003. 2003 Third IEEE Conference on, 1, pages: 56-59, 2003 (inproceedings)

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Atomic force microscope probe based controlled pushing for nano-tribological characterization

Sitti, M.

IEEE/ASME Transactions on Mechatronics, 8(3), 2003 (article)

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Efficient charge recovery method for driving piezoelectric actuators with quasi-square waves

Campolo, D., Sitti, M., Fearing, R. S.

IEEE transactions on ultrasonics, ferroelectrics, and frequency control, 50(3):237-244, IEEE, 2003 (article)

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Synthetic gecko foot-hair micro/nano-structures for future wall-climbing robots

Sitti, M., Fearing, R. S.

In Robotics and Automation, 2003. Proceedings. ICRA’03. IEEE International Conference on, 1, pages: 1164-1170, 2003 (inproceedings)

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[BibTex]


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Piezoelectrically actuated four-bar mechanism with two flexible links for micromechanical flying insect thorax

Sitti, M.

IEEE/ASME transactions on mechatronics, 8(1):26-36, IEEE, 2003 (article)

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Biomimetic propulsion for a swimming surgical micro-robot

Edd, J., Payen, S., Rubinsky, B., Stoller, M. L., Sitti, M.

In Intelligent Robots and Systems, 2003.(IROS 2003). Proceedings. 2003 IEEE/RSJ International Conference on, 3, pages: 2583-2588, 2003 (inproceedings)

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Project Page [BibTex]

Project Page [BibTex]

2000


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Phenomenological damping in optical response tensors

Buckingham, A., Fischer, P.

PHYSICAL REVIEW A, 61(3), 2000 (article)

Abstract
Although perturbation theory applied to the optical response of a molecule or material system is only strictly valid far from resonances, it is often applied to ``near-resonance{''} conditions by means of complex energies incorporating damping. Inconsistent signs of the damping in optical response tensors have appeared in the recent literature, as have errors in the treatment of the perturbation by a static held. The ``equal-sign{''} convention used in a recent publication yields an unphysical material response, and Koroteev's intimation that linear electro-optical circular dichroism may exist in an optically active liquid under resonance conditions is also flawed. We show that the isotropic part of the Pockels tensor vanishes.

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DOI [BibTex]

2000


DOI [BibTex]


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Ab initio investigation of the sum-frequency hyperpolarizability of small chiral molecules

Champagne, B., Fischer, P., Buckingham, A.

CHEMICAL PHYSICS LETTERS, 331(1):83-88, 2000 (article)

Abstract
Using a sum-over-states procedure based on configuration interaction singles /6-311++G{*}{*}, we have computed the sum-frequency hyperpolarizability beta (ijk)(-3 omega; 2 omega, omega) Of two small chiral molecules, R-monofluoro-oxirane and R-(+)-propylene oxide. Excitation energies were scaled to fit experimental UV-absorption data and checked with ab initio values from time-dependent density functional theory. The isotropic part of the computed hyperpolarizabilities, beta(-3 omega; 2 omega, omega), is much smaller than that reported previously from sum-frequency generation experiments on aqueous solutions of arabinose. Comparison is made with a single-centre chiral model. (C) 2000 Elsevier Science B.V. All rights reserved.

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DOI [BibTex]

DOI [BibTex]