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2013


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Hybrid nanocolloids with programmed three-dimensional shape and material composition

Mark, A. G., Gibbs, J. G., Lee, T., Fischer, P.

NATURE MATERIALS, 12(9):802-807, 2013, Max Planck Press Release. (article)

Abstract
Tuning the optical(1,2), electromagnetic(3,4) and mechanical properties of a material requires simultaneous control over its composition and shape(5). This is particularly challenging for complex structures at the nanoscale because surface-energy minimization generally causes small structures to be highly symmetric(5). Here we combine low-temperature shadow deposition with nanoscale patterning to realize nanocolloids with anisotropic three-dimensional shapes, feature sizes down to 20 nm and a wide choice of materials. We demonstrate the versatility of the fabrication scheme by growing three-dimensional hybrid nanostructures that contain several functional materials with the lowest possible symmetry, and by fabricating hundreds of billions of plasmonic nanohelices, which we use as chiral metafluids with record circular dichroism and tunable chiroptical properties.

Max Planck Press Release.

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Video - Fabrication of Designer Nanostructures DOI [BibTex]


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Magnetoelastic coupling in epitaxial cobalt ferrite/barium titanate heterostructures

Gräfe, J., Welke, M., Bern, F., Ziese, M., Denecke, R.

Journal of Magnetism and Magnetic Materials, 339, pages: 84-88, 2013 (article)

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DOI [BibTex]

DOI [BibTex]


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Chiral Colloidal Molecules And Observation of The Propeller Effect

Schamel, D., Pfeifer, M., Gibbs, J. G., Miksch, B., Mark, A. G., Fischer, P.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 135(33):12353-12359, 2013 (article)

Abstract
Chiral molecules play an important role in biological and chemical processes, but physical effects due to their symmetry-breaking are generally weak. Several physical chiral separation schemes which could potentially be useful, including the propeller effect, have therefore not yet been demonstrated at the molecular scale. However, it has been proposed that complex nonspherical colloidal particles could act as ``colloidal molecules{''} in mesoscopic model systems to permit the visualization of molecular phenomena that are otherwise difficult to observe. Unfortunately, it is difficult to synthesize such colloids because surface minimization generally favors the growth of symmetric particles. Here we demonstrate the production of large numbers of complex colloids with glancing angle physical vapor deposition. We use chiral colloids to demonstrate the Baranova and Zel'dovich (Baranova, N. B.; Zel'dovich, B. Y. Chem. Phys. Lett. 1978, 57, 435) propeller effect: the separation of a racemic mixture by application of a rotating field that couples to the dipole moment of the enantiomers and screw propels them in opposite directions. The handedness of the colloidal suspensions is monitored with circular differential light scattering. An exact solution for the colloid's propulsion is derived, and comparisons between the colloidal system and the corresponding effect at the molecular scale are made.

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Video - Nanospropellers DOI [BibTex]

Video - Nanospropellers DOI [BibTex]


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Indirect absorption spectroscopy using quantum cascade lasers: mid-infrared refractometry and photothermal spectroscopy

Pfeifer, M., Ruf, A., Fischer, P.

OPTICS EXPRESS, 21(22):25643-25654, 2013 (article)

Abstract
We record vibrational spectra with two indirect schemes that depend on the real part of the index of refraction: mid-infrared refractometry and photothermal spectroscopy. In the former, a quantum cascade laser (QCL) spot is imaged to determine the angles of total internal reflection, which yields the absorption line via a beam profile analysis. In the photothermal measurements, a tunable QCL excites vibrational resonances of a molecular monolayer, which heats the surrounding medium and changes its refractive index. This is observed with a probe laser in the visible. Sub-monolayer sensitivities are demonstrated. (C) 2013 Optical Society of America

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DOI [BibTex]


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Plasmonic nanohelix metamaterials with tailorable giant circular dichroism

Gibbs, J. G., Mark, A. G., Eslami, S., Fischer, P.

APPLIED PHYSICS LETTERS, 103(21), 2013, Featured cover article. (article)

Abstract
Plasmonic nanohelix arrays are shown to interact with electromagnetic fields in ways not typically seen with ordinary matter. Chiral metamaterials (CMMs) with feature sizes small with respect to the wavelength of visible light are a promising route to experimentally achieve such phenomena as negative refraction without the need for simultaneously negative e and mu. Here we not only show that giant circular dichroism in the visible is achievable with hexagonally arranged plasmonic nanohelix arrays, but that we can precisely tune the optical activity via morphology and lattice spacing. The discrete dipole approximation is implemented to support experimental data. (C) 2013 AIP Publishing LLC.

Featured cover article.

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DOI [BibTex]

DOI [BibTex]


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Quantum cryo-sieving for hydrogen isotope separation in microporous frameworks: an experimental study on the correlation between effective quantum sieving and pore size

Oh, H., Park, K. S., Kalidindi, S. B., Fischer, R. A., Hirscher, M.

{Journal of Materials Chemistry A}, 1, pages: 3244-3248, Royal Society of Chemistry, Cambridge, UK, 2013 (article)

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DOI [BibTex]

DOI [BibTex]


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Gold nanocrystals in high-temperature superconducting films: creation of pinning patterns of choice

Katzer, C., Stahl, C., Michalowski, P., Treiber, S., Schmidl, F., Seidel, P., Albrecht, J., Schütz, G.

{New Journal of Physics}, 15(11), Institute of Physics Pub., Bristol, UK, 2013 (article)

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DOI [BibTex]

DOI [BibTex]


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Theory of scattering of crystal electrons at magnons

Haag, Michael, Illg, C., Fähnle, M.

{Physical Review B}, Published by the American Physical Society through the American Institute of Physics, Woodbury, NYAmerican Institute of Physics, Woodbury, NY, 2013 (article)

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DOI [BibTex]

DOI [BibTex]


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The effect of magnetocrystalline anisotropy on the domain structure of patterned Fe2CrSi Heusler alloy thin films

Miyawaki, T., Foerster, M., Finizio, S., Vaz, C. A. F., Mawass, M.-A., Inagaki, K., Fukatani, N., Le Guyader, L., Nolting, F., Ueda, K., Asano, H., Kläui, M.

{Journal of Applied Physcis}, 114(7), American Institute of Physics, New York, NY, 2013 (article)

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DOI [BibTex]

DOI [BibTex]


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Ion beam lithography for Fresnel zone plates in X-ray microscopy

Keskinbora, K., Grévent, C., Bechtel, M., Weigand, M., Goering, E., Nadzeyka, A., Lloyd, P., Rehbein, S., Schneider, G., Follath, R., Vila-Comamala, J., Yan, H., Schütz, G.

{Optics Express}, 21(10):11747-11756, Optical Society of America, Washington, DC, 2013 (article)

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DOI [BibTex]

DOI [BibTex]


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Is the angular momentum of a ferromagnetic sample after exposure to a fs laser pulse conserved?

Fähnle, M., Haag, M., Illg, C.

{Journal of Magnetism and Magnetic Materials}, 347, pages: 45-46, North-Holland, Amsterdam, 2013 (article)

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DOI [BibTex]

DOI [BibTex]


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Grain boundaries as the controlling factor for the ferromagnetic behaviour of Co-doped ZnO

Straumal, B. B., Mazilkin, A. A., Protasova, S. G., Straumal, P. B., Myatiev, A. A., Schütz, G., Goering, E. J., Tietze, T., Baretzky, B.

{Philosophical Magazine}, 93(10-12):1371-1383, 2013 (article)

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DOI [BibTex]

DOI [BibTex]


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Magnetic properties of electrochemically prepared crystalline films of Prussian blue-based molecular magnets Kj CrIIk [CrIII(CN)6] l \mbox⋅ mH2O

Bhatt, P., Yusuf, S. M., Bhatt, R., Schütz, G.

{Journal of Solid State Electrochemistry}, 17, pages: 1285-1293, Springer-Verlag Germany, 2013 (article)

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DOI [BibTex]

DOI [BibTex]


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H2/D2 adsorption and desorption studies on carbon molecular sieves with different pore structures

Krkljus, I., Steriotis, T., Charalambopoulou, G., Gotzias, A., Hirscher, M.

{Carbon}, 57, pages: 239-247, Elsevier Science, Amsterdam [u.a.], 2013 (article)

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DOI [BibTex]

DOI [BibTex]


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X-ray magnetic circular dichroism strongly influenced by non-magnetic cover layers

Zafar, K., Audehm, P., Schütz, G., Goering, E., Pathak, M., Chetry, K. B., LeClair, P. R., Gupta, A.

{Journal of Electron Spectroscopy and Related Phenomena}, 191, pages: 1-6, Elsevier, Amsterdam, 2013 (article)

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DOI [BibTex]

DOI [BibTex]


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Quantum kinetic theory for demagnetization after femtosecond laser pulses

Teeny, N.

Universität Stuttgart, Stuttgart, 2013 (mastersthesis)

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[BibTex]

[BibTex]


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Exchange bias in La0.7Sr0.3MnO3 / SrMnO3 / La0.7Sr0.3MnO3 trilayers

Jungbauer, M., Hühn, S., Michelmann, M., Goering, E., Moshnyaga, V.

{Journal of Applied Physcis}, 113(17), American Institute of Physics, New York, NY, 2013 (article)

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DOI [BibTex]

DOI [BibTex]


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General decoupling procedure for expectation values of four-operator products in electron-phonon quantum kinetics

Teeny, N., Fähnle, M.

{Journal of Physics A: Mathematical and Theoretical}, 46(38), IOP Pub., London, 2013 (article)

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DOI [BibTex]

DOI [BibTex]


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SPD-induced changes of structure and magnetic properties in the Cu-Co alloys

Straumal, B. B., Protasova, S. G., Mazilkin, A. A., Kogtenkova, O. A., Kurmanaeva, L., Baretzky, B., Schütz, G., Korneva, A., Zieba, P.

{Materials Letters}, 98, pages: 217-221, Elsevier, Amsterdam, 2013 (article)

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DOI [BibTex]

DOI [BibTex]


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Ferromagnetic behaviour of Fe-doped ZnO nanograined films

Straumal, B. B., Protasova, S. G., Mazilkin, A. A., Tietze, T., Goering, E., Schütz, G., Straumal, P. B., Baretzky, B.

{Beilstein Journal of Nanotechnology}, 4, pages: 361-369, 2013 (article)

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DOI [BibTex]

DOI [BibTex]


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The effect of magnetic anisotropy on the spin configurations of patterned La0.7Sr0.3MnO3 elements

Wohlhüter, P., Rhensius, J., Vaz, C. A. F., Heidler, J., Körner, H. S., Bisig, A., Foerster, M., Méchin, L., Gaucher, F., Locatelli, A., Niño, M. A., El Moussaoui, S., Nolting, F., Goering, E., Heyderman, L. J., Kläui, M.

{Journal of Physics: Condensed Matter}, 25, IOP Pub., Bristol, UK, 2013 (article)

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DOI [BibTex]

DOI [BibTex]


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The avalanche process in gold covered MgB2 films

Stahl, C., Treiber, S., Schütz, G., Albrecht, J.

{Superconductor Science and Technology}, 26, IOP Pub., Bristol, 2013 (article)

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DOI [BibTex]

DOI [BibTex]


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MFU-4 - A metal-organic framework for highly effective H2/D2 separation

Teufel, J., Oh, H., Hirscher, M., Wahiduzzaman, M., Zhechkov, L., Kuc, A., Heine, T., Denysenko, D., Volkmer, D.

{Advanced Materials}, 25(4):635-639, Wiley-VCH Verlag, Weinheim, 2013 (article)

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DOI [BibTex]

DOI [BibTex]


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Delayed magnetic vortex core reversal

Kammerer, M., Sproll, M., Stoll, H., Noske, M., Weigand, M., Illg, C., Fähnle, M., Schütz, G.

{Applied Physics Letters}, 102, American Institute of Physics, Melville, NY, 2013 (article)

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DOI [BibTex]

DOI [BibTex]


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Self-organized state formation in magnonic vortex crystals

Adolff, C. F., Hänze, M., Vogel, A., Weigand, M., Martens, M., Meier, G.

{Physical Review B}, 88(22), American Physical Society, Woodbury, NY, 2013 (article)

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DOI [BibTex]

DOI [BibTex]


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Erratum: Generalized Gilbert equation including inertial damping: Derivation from an extended breathing Fermi surface model [Phys. Rev. B 84, 172403 (2011)]

Fähnle, M., Steiauf, D., Illg, C.

{Physical Review B}, 88, American Physical Society, Woodbury, NY, 2013 (article)

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DOI [BibTex]

DOI [BibTex]


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Strain and composition dependence of orbital polarization in nickel oxide superlattices

Wu, M., Benckiser, E., Haverkort, M. W., Franco, A., Lu, J., Nwankwo, U., Brück, S., Audehm, P., Goering, E., Macke, S., Hinkov, V., Wochner, P., Christiani, G., Heinze, S., Logvenov, G., Habermeier, H., Keimer, B.

{Physical Review B}, 88, Published by the American Physical Society through the American Institute of Physics, Woodbury, NY, 2013 (article)

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DOI [BibTex]

DOI [BibTex]


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Efficient focusing of 8 keV X-rays with multilayer Fresnel zone plates fabricated by atomic layer deposition and focused ion beam milling

Mayer, M., Keskinbora, K., Grévent, C., Szeghalmi, A., Knez, M., Weigand, M., Snigirev, A., Snigereva, I., Schütz, G.

{Journal of Synchrotron Radiation}, 20, pages: 433-440, Published for the International Union of Crystallography by Munksgaard, Copenhagen, Denmark, 2013 (article)

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DOI [BibTex]

DOI [BibTex]


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Rapid prototyping of Fresnel zone plates via direct Ga+ ion beam lithography for high-resolution x-ray imaging

Keskinbora, K., Grévent, C., Eigenthaler, U., Weigand, M., Schütz, G.

{ACS Nano}, 7(11):9788-9797, American Chemical Society, Washington, DC, 2013 (article)

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DOI [BibTex]

DOI [BibTex]


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Eine kryoflexible kovalente organische Gerüststruktur für die effiziente Trennung von Wasserstoffisotopien durch Quantensieben

Oh, H., Kalidindi, S. B., Um, Y., Bureekaew, S., Schmid, R., Fischer, R. A., Hirscher, M.

{Angewandte Chemie}, 125(50):13461-13464, Wiley-VCH Verl., Weinheim, 2013 (article)

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DOI [BibTex]

DOI [BibTex]


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Ultrafast demagnetization after laser irradiation in transition metals: Ab initio calculations of the spin-flip electron-phonon scattering with reduced exchange splitting

Illg, C., Haag, M., Fähnle, M.

{Physical Review B}, 88, American Physical Society, Woodbury, NY, 2013 (article)

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DOI [BibTex]

DOI [BibTex]


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Phase diagram for magnetic vortex core switching studied by ferromagnetic absorption spectroscopy and time-resolved transmission x-ray microscopy

Martens, M., Kamionka, T., Weigand, M., Stoll, H., Tyliszczak, T., Meier, G.

{Physical Review B}, 87, Published by the American Physical Society through the American Institute of Physics, Woodbury, NY, 2013 (article)

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DOI [BibTex]

DOI [BibTex]


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Switching modes in easy and hard axis magnetic reversal in a self-assembled antidot array

Haering, F., Wiedwald, U., Nothelfer, S., Koslowski, B., Ziemann, P., Lechner, L., Wallucks, A., Lebecki, K., Nowak, U., Gräfe, J., Goering, E., Schütz, G.

{Nanotechnology}, 24, IOP Pub., Bristol, UK, 2013 (article)

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DOI Project Page [BibTex]

DOI Project Page [BibTex]


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Time-resolved imaging of nonlinear magnetic domain-wall dynamics in ferromagnetic nanowires

Stein, F.-U., Bocklage, L., Weigand, M., Meier, G.

{Scientific Reports}, 3, Nature Publishing Group, London, UK, 2013 (article)

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DOI [BibTex]

DOI [BibTex]


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A cryogenically flexible covalent organic framework for efficient hydrogen isotrope separation by quantum sieving

Oh, H., Kalidindi, S. B., Um, Y., Bureekaew, S., Schmid, R., Fischer, R. A., Hirscher, M.

{Angewandte Chemie International Edition in English}, 52(50):13219-13222, Wiley-VCH Verlag GmbH & Co. KGaA, D-69451 Weinheim, 2013 (article)

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DOI [BibTex]

DOI [BibTex]


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Unexpected room-temperature ferromagnetism in bulk ZnO

Chen, Y., Goering, E., Jeurgens, L., Wang, Z., Phillipp, F., Baier, J., Tietze, T., Schütz, G.

{Applied Physics Letters}, (103), American Institute of Physics, Melville, NY, 2013 (article)

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DOI [BibTex]

DOI [BibTex]


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Large-area hard magnetic L10-FePt and composite L10-FePt based nanopatterns

Goll, D., Bublat, T.

{Physica Status Solidi A-Applications and Materials Science}, 210(7):1261-1271, Wiley-VCH, Weinheim, 2013 (article)

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DOI [BibTex]

DOI [BibTex]


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Wave modes of collective vortex gyration in dipolar-coupled-dot-array magnonic crystals

Han, D., Vogel, A., Jung, H., Lee, K., Weigand, M., Stoll, H., Schütz, G., Fischer, P., Meier, G., Kim, S.

{Scientific Reports}, 3, Nature Publishing Group, London, UK, 2013 (article)

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DOI [BibTex]

DOI [BibTex]


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Ferromagnetism of zinc oxide nanograined films

Straumal, B. B., Protasova, S. G., Mazilkin, A. A., Schütz, G., Goering, E., Baretzky, B., Straumal, P. B.

{Journal of Experimental and Theoretical Physics Letters}, 97(6):367-377, Pleiades Publishing, Inc., 2013 (article)

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DOI [BibTex]

DOI [BibTex]


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Hydrogen adsorption properties of platinum decorated hierarchically structured templated carbons

Oh, H., Gennett, T., Atanassov, P., Kurttepeli, M., Bals, S., Hurst, K. E., Hirscher, M.

{Microporous and Mesoporous Materials}, pages: 66-74, Elsevier, Amsterdam, 2013 (article)

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DOI [BibTex]

DOI [BibTex]


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Extended s-d models for the dynamics of noncollinear magnetization: Short review of two different approaches

Fähnle, M., Zhang, S.

{Journal of Magnetism and Magnetic Materials}, 326, pages: 232-234, NH, Elsevier, Amsterdam, 2013 (article)

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DOI [BibTex]

DOI [BibTex]


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Correlation between spin structure oscillations and domain wall velocities

Bisig, A., Stärk, M., Mawass, M., Moutafis, C., Rhensius, J., Heidler, J., Büttner, F., Noske, M., Weigand, M., Eisebitt, S., Tyliszczak, T., Van Wayenberge, B., Stoll, H., Schütz, G., Kläui, M.

{Nature Communications}, 4, Nature Publishing Group, London, 2013 (article)

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DOI [BibTex]

DOI [BibTex]


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Recent advances in use of atomic layer deposition and focused ion beams for fabrication of Fresnel zone plates for hard x-rays

Keskinbora, K., Robisch, A., Mayer, M., Grévent, C., Szeghalmi, A. V., Knez, M., Weigand, M., Snigireva, I., Snigirev, A., Salditt, T., Schütz, G.

{Proceedings of SPIE (The International Society for Optical Engineering)}, 8851, 2013 (article)

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DOI [BibTex]

DOI [BibTex]


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Magnetic states in low-pinning high-anisotropy material nanostructures suitable for dynamic imaging

Büttner, F., Moutafis, C., Bisig, A., Wohlhüter, P., Günther, C. M., Mohanty, J., Geilhufe, J., Schneider, M., v. Korff Schmising, C., Schaffert, S., Pfau, B., Hantschmann, M., Riemeier, M., Emmel, M., Finizio, S., Jakob, G., Weigand, M., Rhensius, J., Franken, J. H., Lavrijsen, R., Swagten, H. J. M., Stoll, H., Eisebitt, S., Kläui, M.

{Physical Review B}, 87, Published by the American Physical Society through the American Institute of Physics, Woodbury, NY, 2013 (article)

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DOI [BibTex]

DOI [BibTex]


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Experimental and theoretical study of D2/H2 quantum sieving in a carbon molecular sieve

Gotzias, A., Charalambopoulou, G., Ampoumogli, A., Krkljus, I., Hirscher, M., Steriotis, T.

{Adsorption}, 19(2-4):373-379, Springer Science+Business Media, New York, 2013 (article)

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DOI [BibTex]

DOI [BibTex]

2011


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Quantum-Cascade Laser-Based Vibrational Circular Dichroism

Luedeke, S., Pfeifer, M., Fischer, P.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 133(15):5704-5707, 2011 (article)

Abstract
Vibrational circular dichroism (VCD) spectra were recorded with a tunable external-cavity quantum-cascade laser (QCL). In comparison with standard thermal light sources in the IR, QCLs provide orders of magnitude more power and are therefore promising for VCD studies in strongly absorbing solvents. The brightness of this novel light source is demonstrated with VCD and IR absorption measurements of a number of compounds, including proline in water.

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DOI [BibTex]

2011


DOI [BibTex]


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Actively coupled cavity ringdown spectroscopy with low-power broadband sources

Petermann, C., Fischer, P.

OPTICS EXPRESS, 19(11):10164-10173, 2011 (article)

Abstract
We demonstrate a coupling scheme for cavity enhanced absorption spectroscopy that makes use of an intracavity acousto-optical modulator to actively switch light into (and out of) a resonator. This allows cavity ringdown spectroscopy (CRDS) to be implemented with broadband nonlaser light sources with spectral power densities of less than 30 mu W/nm. Although the acousto-optical element reduces the ultimate detection limit by introducing additional losses, it permits absorptivities to be measured with a high dynamic range, especially in lossy environments. Absorption measurements for the forbidden transition of gaseous oxygen in air at similar to 760nm are presented using a low-coherence cw-superluminescent diode. The same setup was electronically configured to cover absorption losses from 1.8 x 10(-8)cm(-1) to 7.5\% per roundtrip. This could be of interest in process analytical applications. (C) 2011 Optical Society of America

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DOI [BibTex]

DOI [BibTex]


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Magnetically actuated propulsion at low Reynolds numbers: towards nanoscale control

Fischer, P., Ghosh, A.

NANOSCALE, 3(2):557-563, 2011 (article)

Abstract
Significant progress has been made in the fabrication of micron and sub-micron structures whose motion can be controlled in liquids under ambient conditions. The aim of many of these engineering endeavors is to be able to build and propel an artificial micro-structure that rivals the versatility of biological swimmers of similar size, e. g. motile bacterial cells. Applications for such artificial ``micro-bots'' are envisioned to range from microrheology to targeted drug delivery and microsurgery, and require full motion-control under ambient conditions. In this Mini-Review we discuss the construction, actuation, and operation of several devices that have recently been reported, especially systems that can be controlled by and propelled with homogenous magnetic fields. We describe the fabrication and associated experimental challenges and discuss potential applications.

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Video - Nanospropellers DOI [BibTex]


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The Oxidation of Fe(111)

Davies, R., Edwards, D., Gräfe, J., Gilbert, L., Davies, P., Hutchings, G., Bowker, M.

Surface Science, 605(17-18):1754-1762, 2011 (article)

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DOI [BibTex]

DOI [BibTex]